Physics:Ultracold neutrons

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Short description: Free neutrons stored in very small traps


Ultracold neutrons (UCN) are free neutrons which can be stored in traps made from certain materials. The storage is based on the reflection of UCN by such materials under any angle of incidence.

Properties

The reflection is caused by the coherent strong interaction of the neutron with atomic nuclei. It can be quantum-mechanically described by an effective potential which is commonly referred to as the Fermi pseudo potential or the neutron optical potential. The corresponding velocity is called the critical velocity of a material. Neutrons are reflected from a surface if the velocity component normal to the reflecting surface is less than or equal to the critical velocity.

As the neutron optical potential of most materials is below 300 neV, the kinetic energy of incident neutrons must not be higher than this value to be reflected under any angle of incidence, especially for normal incidence. The kinetic energy of 300 neV corresponds to a maximum velocity of 7.6 m/s or a minimum wavelength of 52 nm. As their density is usually very small, UCN can also be described as a very thin ideal gas with a temperature of 3.5 mK. Moreover, materials with a high optical potential (~ 1 µeV) are used for the design of cold neutrons optical components.[1]

Due to the small kinetic energy of an UCN, the influence of gravitation is significant. Thus, the trajectories are parabolic. Kinetic energy of an UCN is transformed into potential (height) energy with ~102 neV/m.

The magnetic moment of the neutron, produced by its spin, interacts with magnetic fields. The total energy changes with ~60 neV/T.

History

It was Enrico Fermi who realized first that the coherent scattering of slow neutrons would result in an effective interaction potential for neutrons traveling through matter, which would be positive for most materials.[2] The consequence of such a potential would be the total reflection of neutrons slow enough and incident on a surface at a glancing angle. This effect was experimentally demonstrated by Fermi and Walter Henry Zinn[3] and Fermi and Leona Marshall.[4] The storage of neutrons with very low kinetic energies was predicted by Yakov Borisovich Zel'dovich[5] and experimentally realized simultaneously by groups at Dubna[6] and Munich.[7]

UCN production

There are various methods for the production of UCN. Such facilities have been built and are in operation:

  1. The use of a horizontal evacuated tube from the reactor, curved so all but UCN would be absorbed by the walls of the tube before reaching the detector.[6]
  2. Neutrons transported from the reactor though a vertical evacuated guide about 11 meters long are slowed down by gravity, so only those that happened to have ultracold energies can reach the detector at the top of the tube.[7]
  3. A neutron turbine in which neutrons at 50 m/s are directed against the blades of a turbine wheel with receding tangential velocity 25 m/s, from which neutrons emerge after multiple reflections with a speed of about 5 m/s.[8][9][10]
  4. After protons are accelerated to around 600 MeV they impinge on a lead target and produce neutrons via spallation. These neutrons are thermalized in e.g. heavy water and then moderated e.g. in liquid or solid deuterium to be cold. The final production of UCN occurs via downscattering in solid deuterium. Such a UCN source[11] was realized at the Paul Scherrer Institute, Switzerland and at the Los Alamos National Laboratory, USA.

Reflecting materials

Material: VF[12] vC[13] η (10−4)[13]
Beryllium 252 neV 6.89 m/s 2.0–8.5
BeO 261 neV 6.99 m/s
Nickel 252 neV 6.84 m/s 5.1
Diamond 304 neV 7.65 m/s
Graphite 180 neV 5.47 m/s
Iron 210 neV 6.10 m/s 1.7–28
Copper 168 neV 5.66 m/s 2.1–16
Aluminium 054 neV 3.24 m/s 2.9–10

Any material with a positive neutron optical potential can reflect UCN. The table on the right gives an (incomplete) list of UCN reflecting materials including the height of the neutron optical potential (VF) and the corresponding critical velocity (vC). The height of the neutron optical potential is isotope-specific. The highest known value of VF is measured for 58Ni: 335 neV (vC = 8.14 m/s). It defines the upper limit of the kinetic energy range of UCN.

The most widely used materials for UCN wall coatings are beryllium, beryllium oxide, nickel (including 58Ni) and more recently also diamond-like carbon (DLC).

Non-magnetic materials such as DLC are usually preferred for the use with polarized neutrons. Magnetic centers in e.g. Ni can lead to de-polarization of such neutrons upon reflection. If a material is magnetized, the neutron optical potential is different for the two polarizations, caused by

[math]\displaystyle{ V_F(pol.)=V_F(unpol.)\pm\mu_N\cdot B }[/math]

where [math]\displaystyle{ \mu_N }[/math] is the magnetic moment of the neutron and [math]\displaystyle{ B=\mu_0\cdot M }[/math] the magnetic field created on the surface by the magnetization.

Each material has a specific loss probability per reflection,

[math]\displaystyle{ \mu(E,\theta)=2\eta\sqrt{\frac{E\cos^2\theta}{V_F-E\cos^2\theta}} }[/math]

which depends on the kinetic energy of the incident UCN (E) and the angle of incidence (θ). It is caused by absorption and thermal upscattering. The loss coefficient η is energy-independent and typically of the order of 10−4 to 10−3.

Experiments with UCN

The production, transportation and storage of UCN is currently motivated by their usefulness as a tool to determine properties of the neutron and to study fundamental physical interactions. Storage experiments have improved the accuracy or the upper limit of some neutron related physical values.

Measurement of the neutron lifetime

Today's world average value for the neutron lifetime is [math]\displaystyle{ 885.7\pm0.8\,{\mathrm s}\, }[/math],[14] to which the experiment of Arzumanov et al.[15] contributes strongest. Ref.[15] measured [math]\displaystyle{ \tau_n=885.4\pm0.9_{\mathrm{stat}}\pm0.4_{\mathrm{syst}}\,{\mathrm s}\, }[/math] by storage of UCN in a material bottle covered with Fomblin oil (perfluoropolyether vacuum oil)). Using traps with different surface to volume ratios allowed them to separate storage decay time and neutron lifetime from each other. There is another result, with even smaller uncertainty, but which is not included in the World average. It was obtained by Serebrov et al.,[16] who found [math]\displaystyle{ 878.5~\pm0.7_{\mathrm{stat}}\pm0.4_{\mathrm{syst}}\,{\mathrm s}\, }[/math]. Thus, the two most precisely measured values deviate by 5.6 σ.

Measurement of the neutron electric dipole moment

Main page: Physics:Neutron electric dipole moment

The neutron electric dipole moment is a measure for the distribution of positive and negative charge inside the neutron. No neutron electric dipole moment has been found as of October 2019). The lowest value for the upper limit of the neutron electric dipole moment was measured with stored UCN (see main article).

Observation of the gravitational interactions of the neutron

Physicists have observed quantized states of matter under the influence of gravity for the first time. Valery Nesvizhevsky of the Institut Laue-Langevin and colleagues found that cold neutrons moving in a gravitational field do not move smoothly but jump from one height to another, as predicted by quantum theory. The finding could be used to probe fundamental physics such as the equivalence principle, which states that different masses accelerate at the same rate in a gravitational field (V Nesvizhevsky et al. 2001 Nature 415 297). UCN spectroscopy has been used to limit scenarios including dark energy, chameleon fields,[17] and new short range forces.[18]

Search for Neutron to Mirror-Neutron Oscillations

see Mirror Matter

Measurement of the neutron-anti-neutron oscillation time

Measurement of the A-coefficient of the neutron beta decay correlation

The first reported measurement of the beta-asymmetry using UCN is from a Los Alamos group in 2009.[19] The LANSCE group published precision measurements with polarized UCN the next year.[20] Further measurements by these groups and others have led to the current world average:[21]

[math]\displaystyle{ A_0 = -0.1184 \pm 0.0010 }[/math]

References

  1. ↑ Hadden, Elhoucine; Iso, Yuko; Kume, Atsushi; Umemoto, Koichi; Jenke, Tobias; Fally, Martin; Klepp, Jürgen; Tomita, Yasuo (2022-05-24). "Nanodiamond-based nanoparticle-polymer composite gratings with extremely large neutron refractive index modulation". Photosensitive Materials and their Applications II. 12151. SPIE. pp. 70–76. doi:10.1117/12.2623661. ISBN 9781510651784. Bibcode: 2022SPIE12151E..09H. https://www.spiedigitallibrary.org/conference-proceedings-of-spie/12151/1215109/Nanodiamond-based-nanoparticle-polymer-composite-gratings-with-extremely-large-neutron/10.1117/12.2623661.full. 
  2. ↑ E. Fermi, Ricerca Scientifica 7 (1936) 13
  3. ↑ Anonymous (1946). "Minutes of the Meeting at Chicago, June 20-22, 1946". Physical Review 70 (1–2): 99. doi:10.1103/PhysRev.70.99. Bibcode: 1946PhRv...70...99.. 
  4. ↑ Fermi, E.; Marshall, L. (1947-05-15). "Interference Phenomena of Slow Neutrons". Physical Review (American Physical Society (APS)) 71 (10): 666–677. doi:10.1103/physrev.71.666. ISSN 0031-899X. Bibcode: 1947PhRv...71..666F. 
  5. ↑ Zeldovich, Ya.B. (1959). "Storage of cold neutrons". Soviet Physics Journal of Experimental& Theoretical Physics 9: 1389. 
  6. ↑ 6.0 6.1 V.I. Lushikov et al., Sov. Phys. JETP Lett. 9 (1969) 23
  7. ↑ 7.0 7.1 Steyerl, A. (1969). "Measurements of total cross sections for very slow neutrons with velocities from 100 m/sec to 5 m/sec". Physics Letters B 29 (1): 33–35. doi:10.1016/0370-2693(69)90127-0. Bibcode: 1969PhLB...29...33S. 
  8. ↑ A. Steyerl; H. Nagel; F.-X. Schreiber; K.-A. Steinhauser; R. Gähler; W. Gläser; P. Ageron; J. M. Astruc et al. (1986). "A new source of cold and ultracold neutrons". Phys. Lett. A 116 (7): 347–352. doi:10.1016/0375-9601(86)90587-6. Bibcode: 1986PhLA..116..347S. https://dx.doi.org/10.1016/0375-9601%2886%2990587-6. 
  9. ↑ "ILL Yellow Book". https://www.ill.eu/users/instruments/instruments-list/pf2/selected-highlights/the-search-for-a-neutron-electric-dipole-moment. 
  10. ↑ Stefan Döge; Jürgen Hingerl; Christoph Morkel (Feb 2020). "Measured velocity spectra and neutron densities of the PF2 ultracold-neutron beam ports at the Institut Laue–Langevin". Nucl. Instrum. Methods A 953: 163112. doi:10.1016/j.nima.2019.163112. Bibcode: 2020NIMPA.95363112D. http://www.sciencedirect.com/science/article/pii/S0168900219314445. 
  11. ↑ Lauss, Bernhard; Blau, Bertrand (2021-09-06). "UCN, the ultracold neutron source -- neutrons for particle physics" (in en). SciPost Physics Proceedings (5): 004. doi:10.21468/SciPostPhysProc.5.004. ISSN 2666-4003. https://scipost.org/SciPostPhysProc.5.004. 
  12. ↑ R. Golub, D. Richardson, S.K. Lamoreaux, Ultra-Cold Neutrons, Adam Hilger (1991), Bristol
  13. ↑ 13.0 13.1 V.K. Ignatovich, The Physics of Ultracold Neutrons, Clarendon Press (1990), Oxford, UK
  14. ↑ al, W-M Yao (2006-07-01). "Review of Particle Physics". Journal of Physics G: Nuclear and Particle Physics 33 (1): 1–1232. doi:10.1088/0954-3899/33/1/001. ISSN 0954-3899. Bibcode: 2006JPhG...33....1Y.  and 2007 partial update for edition 2008 (URL: http://pdg.lbl.gov)
  15. ↑ 15.0 15.1 Arzumanov, S; Bondarenko, L; Chernyavsky, S; Drexel, W; Fomin, A et al. (2000). "Neutron life time value measured by storing ultracold neutrons with detection of inelastically scattered neutrons". Physics Letters B (Elsevier BV) 483 (1–3): 15–22. doi:10.1016/s0370-2693(00)00579-7. ISSN 0370-2693. Bibcode: 2000PhLB..483...15A. 
  16. ↑ Serebrov, A.; Varlamov, V.; Kharitonov, A.; Fomin, A.; Pokotilovski, Yu. et al. (2005). "Measurement of the neutron lifetime using a gravitational trap and a low-temperature Fomblin coating". Physics Letters B 605 (1–2): 72–78. doi:10.1016/j.physletb.2004.11.013. ISSN 0370-2693. PMID 27308146. Bibcode: 2005PhLB..605...72S. 
  17. ↑ Jenke, T.; Cronenberg, G.; Burgdörfer, J.; Chizhova, L. A.; Geltenbort, P.; Ivanov, A. N.; Lauer, T.; Lins, T. et al. (16 April 2014). "Gravity Resonance Spectroscopy Constrains Dark Energy and Dark Matter Scenarios". Physical Review Letters 112 (15): 151105. doi:10.1103/PhysRevLett.112.151105. PMID 24785025. Bibcode: 2014PhRvL.112o1105J. 
  18. ↑ Kamiya, Y.; Itagaki, K.; Tani, M.; Kim, G. N.; Komamiya, S. (22 April 2015). "Constraints on New Gravitylike Forces in the Nanometer Range". Physical Review Letters 114 (16): 161101. doi:10.1103/PhysRevLett.114.161101. PMID 25955041. Bibcode: 2015PhRvL.114p1101K. 
  19. ↑ Pattie, R. W.; Anaya, J.; Back, H. O.; Boissevain, J. G.; Bowles, T. J.; Broussard, L. J.; Carr, R.; Clark, D. J. et al. (5 January 2009). "First Measurement of the Neutron β Asymmetry with Ultracold Neutrons". Physical Review Letters 102 (1): 012301. doi:10.1103/PhysRevLett.102.012301. PMID 19257182. Bibcode: 2009PhRvL.102a2301P. http://authors.library.caltech.edu/14811/1/PATprl09.pdf. 
  20. ↑ Liu, J.; Mendenhall, M. P.; Holley, A. T.; Back, H. O.; Bowles, T. J.; Broussard, L. J.; Carr, R.; Clayton, S. et al. (Jul 2010). "Determination of the Axial-Vector Weak Coupling Constant with Ultracold Neutrons". Physical Review Letters 105 (18): 181803. doi:10.1103/PhysRevLett.105.181803. PMID 21231098. Bibcode: 2010PhRvL.105r1803L. 
  21. ↑ K.A. Olive et al. (Particle Data Group) (2014). e−Asymmetry Parameter A. http://pdg8.lbl.gov/rpp2014v1/pdgLive/DataBlock.action?node=S017BA. 



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